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Zaatari, Jordan (CNN) -- Hoping her celebrity will bring attention to the widening Syrian refugee crisis, actress and U.N. envoy Angelina Jolie spoke of the horrors that children, many of them orphans, have witnessed in Syria.

"Body parts separated, and burned people being pulled apart like chicken -- a little 9-year-old girl said that," Jolie said during her visit to a refugee tent camp in Jordan near the Syrian border.

Every day, an estimated 2,000 Syrians are fleeing the relentless bloodshed that has gripped their country for the past 18 months, the United Nations' refugee agency said Tuesday. That adds up to more than a quarter million Syrian refugees -- 253,000 -- now living in camps and other temporary homes inside Jordan, Turkey, Lebanon, and Iraq.

U.N. breakdown of refugees

Life in the dusty Zaatari refugee camp outside Mafraq, Jordan, is not easy for those living there, many of whom have almost nothing after leaving their homes amid violence. Members of one family told CNN they had fled over the border with a 4-day-old baby and the clothes on their backs. Others complained of being short of food and water.

Life in Syrian refugee camps

Tracey Shelton, a senior correspondent for Global Post, was embedded with a group of rebel fighters in Aleppo, Syria, last week when they were hit by a unexpected attack. These seven images from the video she was shooting show the instant of the explosion. The images and Shelton's description of the events were originally published on Global Post. From left, Issa Aiash, 30, his younger brother Ahmed, 17, and Sheihk Mamoud, 42, laugh and joke as they clean their post Saturday, September 8.

The men recieve a call that tanks are nearby. They trade their brooms for weapons.

This frame shows the moment the tank blast hit.

Shelton told Global Post that the blast filled the area with debris and smoke, and left her and her camera covered in dust.

Only one member of the rebel team survived.

The sole survivor checks his injuries.

Shelton says it took several minutes for the dust to clear. They checked for other survivors but found none.

Instant of impact in Aleppo

Instant of impact in Aleppo

Instant of impact in Aleppo

Instant of impact in Aleppo

Instant of impact in Aleppo

Instant of impact in Aleppo

Instant of impact in Aleppo

Instant of impact in Aleppo

Syria accused of using 'barrel bombs'

Escorted to the border overnight by the Jordanian military, Jolie witnessed the moment when Syrians crossed into Jordan, becoming refugees before her eyes. The actress, who is raising six children with partner Brad Pitt, said she was greatly moved by what she had seen and spoke of the connection she felt in particular with the mothers and their children as they faced such challenging times.

"The amount of innocent children that have been reported dead, the amount of innocent children I've met here who are wounded and unaccompanied -- with their parents being killed and now they're on their own -- it's impossible to imagine any mother standing by and not stepping up and doing something to prevent this," she said.

Jolie has made countless trips to the world's hotspots in her role as a U.N. goodwill ambassador -- including a visit to Syrian refugees in Turkey last year.

Jordan is bearing the brunt of the refugee crisis sparked by Syria's civil war: More than 85,000 refugees have escaped to Jordan, and many more have fled to neighboring Turkey, Lebanon and Iraq.

"Jordan has already reached its limit in absorbing the refugee influx, and what is needed now is to build more refugee camps for the Syrian refugees," Jordanian Foreign Minister Nasser Judeh said. "We have limited means, but this is the land of the good people, and we will share with them whatever we have, no matter how little (it) is."

Jolie urged other countries to do more to help the Syrian people.

"I am grateful to Jordan and the border countries for saving the lives (of those) who are dying in Syria. It's an extraordinary thing. We encourage the international community to support the people here until one day they go back home."

In other developments Tuesday:

Diplomacy: U.N. envoy set to meet Al-Assad

Veteran diplomat Lakhdar Brahimi, who was recently appointed the U.N. and Arab League envoy to Syria, will "soon" meet Syrian President Bashar al-Assad, U.N. Secretary General Ban Ki-moon said.

Za'atari Refugee camp in northern Jordan, about six miles from the Syrian border, currently hosts over 20,000 Syrian refugees. UNICEF predicts 70,000 people will be living there by the end of the year.

The pace of new arrivals to the camp has more than doubled in recent weeks, with over 14,000 arriving in the past seven days. Last week an average of 600 people were arriving each day.

The camp was opened less than a month ago to accommodate the growing number of refugees arriving in Jordan since the Syrian uprising began 18 months ago.

Refugees walk at the camp.

A Syrian refugee bathes his child. Water is provided several times daily by water trucks, but supplies of fresh water are very limited and the needs of the refugees are putting pressure on local communities which already experience water shortages.

Clothes hang to dry after being washed.

Nearly half of the camp's residents are children, and there are few activities for them in the camp. Sandstorms often force children to stay inside their tents for long periods of time.

Last month, United Nations humanitarian chief Valerie Amos offered a grim account of the civil war's toll: more than a million people uprooted, a million more in need of urgent aid.

Syrian refugees walk through the camp.

A handicapped Syrian refugee looks out of his tent. Za'atari Camp was built on a barren desert plain without a tree or shrub in sight. Severe sandstorms and scorching heat have taken their toll on refugees and aid workers here.

Syrian refugees look out from their tent.

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Life inside a Syrian refugee camp

Kofi Annan on confronting Assad's lies

Syria's children caught in conflict

It's the latest international diplomatic effort to resolve the ongoing fighting that has claimed more than 20,000 lives over the past year and a half, according to Ban. Brahimi took the place of former U.N. envoy Kofi Annan, who resigned from the post last month after a failed peace deal with Syria. Annan met with al-Assad during his peace efforts.

Brahimi has acknowledged that he faces an uphill struggle, saying he is "fully aware" that his mission is "extremely difficult." He expects to travel to Damascus in the next few days, he said.

Analysis: Al Qaeda looks to Syria to revive its fortunes

Humanitarian crisis: A quarter of Homs residents need aid

The humanitarian situation in Homs is "grave and continues to deteriorate," according to a team of international health experts who visited the embattled province last week as part of a U.N. exploratory mission.

Some 550,000 of the 2.2 million people in the province are in need of humanitarian aid, said World Health Organization spokesman Tarik Jasarevic. And there is little time to get that aid into Homs, which has been a bastion of anti-government sentiment in the Syrian civil war.

"The urgency of scaling up delivery of humanitarian aid is exacerbated by the approaching winter," Jasarevic said.

About half of the province's medical doctors have left, and only about three surgeons remain, he said. Facilities across the province have been damaged or destroyed, leaving only a fraction of the existing hospitals overwhelmed with patients and short on medicine and supplies.

Photographer captures Syria's rebels, escapes death

On the ground: Damascus, Aleppo take another beating

Opposition activists reported a wave of fresh violence in Syria that claimed at least 72 lives nationwide, 30 of them in aerial shelling, according to the opposition Local Coordination Committees of Syria.

Among the deaths were 22 in Aleppo province, where a bakery in Marea was shelled, the LCC said. Syrian regime forces have previously attacked bread lines in the province, according to human rights groups and U.N. officials.

Damascus and its suburbs also saw at least 20 deaths Tuesday. Fierce clashes between regime forces and rebels and heavy gunfire were reported by the LCC, as well as shelling of farms and residential areas.

In Elfaya, in Hama province, the opposition network reports what it describes as a "new massacre" by regime forces, with eight people seized from their farms and executed. Four more are missing, the LCC said.

In Homs, regime forces renewed heavy shelling by tanks and mortars, the LCC said. And in Daraa, the birthplace of demonstrations against President Bashar al-Assad last year, the group reported "heavy and indiscriminate gunfire by regime forces."

State-run media, meanwhile, reported Tuesday that 30 civilians were killed in a "terrorist bombing" Monday in front of an Aleppo hospital. The government said children were among those killed.

Baby survives as family dies in onslaught

CNN's Sara Sidner, Holly Yan, Kareem Khadder, Arwa Damon, Karen Smith and Saskya Vandoorne contributed to this report.